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The records of the Principal's Office, King's College London, comprise minutes, correspondence and memoranda, 1863-1997. These notably include minutes of the Delegacy of King's College School of Medicine and Dentistry, 1989-1990, and various committee minutes including those of the Health and Welfare Committee, Joint Medical Advisory Committee and the Committee for the London Institutes for Advanced Study, 1974-1990; a run of general correspondence relating to College business including staff salaries, property, events, scholarships and relations with other universities, 1944-1979; but also more specifically, personal correspondence with Principal Richard William Jelf, 1863-1864; correspondence and papers on quinquennia and outlining the strategic direction of the College and constituent academic departments, including merger negotiations and the College Charter, 1933-1992; Principal's files relating to named departments, faculties and schools, including the United Medical and Dental Schools Merger, 1988-1997; correspondence on students including named individuals, the Student's Union and some pass lists, 1946-1979; correspondence concerning staff appointments, including professorial and other senior vacancies such as Secretaryship and Principalship, individual Chairs, salary scales, sabbaticals and staff-student relations, 1920-1997, correspondence concerning scholarships and awards, 1988-1997; papers relating to College property including proposals for the redevelopment of the College in Bloomsbury, expansion into Somerset House, Strand, and student residences, 1920-1985; minutes and correspondence concerning College libraries including the Ronald Burrows Memorial Library, 1931- 1977; correspondence and papers on the management of the Liddell Hart Centre for Military Archives, including with donors, 1977-1994; correspondence concerning hospitality and entertainment including Fellows' dinners and graduations, public and inaugural lectures, orations, royal visits and student events, 1946-1997; correspondence and papers charting the relationship of King's with the federal University of London, including Heads of Schools and reports on teaching, post-war reconstruction and the future of Goldsmith's College, 1943-1987; assorted memoranda, 1896-1978.

The records of King's College London Library consist of committee minutes, correspondence, memoranda and other papers, 1830-1998. These include the principal Library Committee minutes and correspondence , 1871-1994; Library Resources Co-ordinating Committee (LRCC) minutes and papers, 1974-1993; Library Services Management Team papers, 1990-1994; minutes of the Strand Campus Users Committee, 1987-1990; minutes, correspondence, reports and memoranda concerning the strategic planning and general policy of the Library including Library Reports, 1987-1990, quinquennia, the University Grants Committee, building, mergers, individual campus libraries committee minutes and overall Library aims and objectives, 1925-1994; papers relating to grants, expenditure and finance, including invoices, 1933-1993; general papers concerning the day-to-day management of the Library including constituent libraries, Second World War disruption, security issues, noise, user/reader services, information retrieval and cataloguing, rare books and Special Collections, policy on periodical subscription, binding and repair, interlibrary loans, publicity and relations with the Students' Union, 1932-1995; correspondence with departments, faculties and schools concerning accessioning policies, 1934-1992; register of borrowers, 1845-1854, 1962-1968, and general correspondence with readers, 1946-1993; papers relating to Library equipment including automation, 1986-1992; papers on building and planning, including the Library Planning and Accommodation Sub-committee, notes on Strand libraries, Cornwall House, Manresa Road, Chelsea, and Hampstead sites, 1948-1993; papers relating to staff and staffing levels, including lists, appointments, appraisals, questionnaires, staff meeting minutes and establishment papers, 1933-1997; individual personnel records of Library staff, 1957-1998; manuscript and typescript Library catalogues and shelf lists, including the Marsden Library, 1830-1993; papers relating to stock, including stock checks and transfers, 1989-1994, accessions registers, 1847, 1932-1975, correspondence and registers of gifts and bequests, including the private papers of academics, 1898-1992, indexes to journals and serials, 1931-[1963]; 1986-1992; papers of Hedwig Pollock, rare book librarian, 1943-1967, including professional correspondence, detailed descriptions of very rare books and manuscript texts and some fragments from a 16th century volume; papers relating to the Liddell Hart Centre for Military Archives and Library, including correspondence with Trustees, minutes of the Trustees and external funding, 1959-1996; interlibrary co-operation and computerised data collection and librarianship including the Standing Conference of Librarians of Libraries of the University of London, Consortium of University Research Libraries (CURL), British Library Research and Development Department, Monitoring and Assessment Research Centre (MARC), Arts and Humanities Data Service (AHDS), European Union Trans-European Mobility Scheme for University Studies (TEMPUS) and Standing Conference of National and University Libraries (SCONUL), 1955-1998.

Chelsea College Library records, 1895-1987, comprise papers collected by the College Library or describing the work of the Library on the Chelsea campus following the merger with King's College in 1985, notably correspondence with the College Secretary and departments, 1974-1980; papers relating to Library computerisation, 1979-1987; staffing and salary matters, 1978-1985; University Grants Committee papers on libraries, 1974-1982; History and Philosophy of Science Library correspondence and bibliography, 1964-1987; Chelsea Campus Libraries Users Committee notes, 1985-1987; finance, 1975-1977; concerning the College History Collection, 1965-1974; notes relating to building and planning at the King's Road site, 1971-1987; University of London merger and other papers, 1978-1983; reports on medical education in London, 1980; concerning Library private papers, 1949-1970; Library Annual Reports, 1963-1987 (1992/CAL, CAL/1986); correspondence concerning Library donors and Zoology reprints, 1967-1985 (Ref: 1986/CAL); accessions registers, 1921-1975 (Ref: CAL/RG); lists of current periodicals, 1960-1974 (Ref: CAL/RGJ); payments books for stock, equipment and expenses, 1960-1973 (Ref: CAL/CB); Library staff personnel files for leavers between 1970-1976 (Ref: CAL/FP); material concerning the history of the College accumulated by the Library, including charters, official reports, with some press cuttings, 1914-1981 (Ref: CAL/H).