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The papers of Kathleen and Millicent Coleman comprise three classes of material: the private papers of the sisters and the Coleman family, 1842-1957; records relating to the National Children's Home, 1935-1981 largely CLOSED; and the Pestalozzi Village Trust, 1948-1989. Personal papers include a diary and pharmacopoeias, correspondence, examination certificates, photographs and printed books, 1842-1957, notably including a detailed manuscript medical diary describing life on board ship and a medical practice in Africa, 1842-1844, probably compiled by John Albert Sidney Coleman, grandfather of Kathleen and Millicent Coleman; pharmacopoeias containing remedies and prescriptions, with printed pharmacopoeias, compiled by Mark Coleman and others, reflecting the transition of the Coleman family business from patent remedies to modern pharmacy, 1851-1894; correspondence with Kathleen and Millicent Coleman, mainly descriptions of daily life in the National Children's Home and describing psychological testing of the children, 1927-1948 (CLOSED); family correspondence and legal documents including letting agreements and deeds of partnership, the will of Mathew Coleman, the sisters' great uncle, and relating to their father and his career, letters containing family news and gossip, 1845-1928; examination certificates and prize lists relating to the education of Kathleen and Millicent Coleman, 1922-1933; photographs of the Coleman family during the 1890s, during World War One and of Kathleen and Millicent Coleman on holiday, [1928], of Lady Eleanor Holles School, 1921-1933, group photographs of students and staff in King's College London Department of History, 1929-1955, photographs of various National Children's Home establishments, 1934-1957; a small collection of printed books concerned with the history, customs and government of London and the Home Counties, [1945-1985] (Boxes 70-74, now on open access in the Archive reading room).

The CLOSED records of the National Children's Home, 1935-1981, notably comprising Vocational Guidance Record Sheets, consisting of files on individual children that included intelligence test results, memory tests and individual comments, arranged in alphabetical order, 1938-1964 (Boxes 1-23); test results and evaluations of named children for tests organised by the National Institute of Industrial Psychology including the Porteus Maze Test and scoring sheets, 1957-1960 (Boxes 24-28); psychological evaluations of children at different branches of the children's home, notably in Cardiff, Harpenden, Nottingham and Glasgow, including individual test results and assessments with broad statistics and educational recommendations by visitors, 1942-1963 (Boxes 29-40); pupil record cards containing biographical information, aptitude tests and psychological test results for children at various homes, [1948-1960] (Boxes 41-42); material relating to the Brentwood College of Education including a working party on syllabuses, staff lists, the relationship with the University of London Institute of Education, manuscript notes and some psychological test results of children engaged in the so-called Gifted Child Study, 1971-1974 (Boxes 43-44); material relating to vocational aptitude and the placement of older children in trades and professions such as the armed forces and Civil Service, notably including psychologists' reports, 1935-1965 (Boxes 45-56); questionnaires of 18 year-old former residents conducted in 1954-1956 (Box 57); material relating to European refugees resident in the NCH including named children and correspondence with the Central Committee for Refugees, 1942-1949 (Boxes 58-59); general correspondence with Millicent Coleman relating to local authorities, staff and the emigration of children to Australia, 1951-1962; manuscript visitation report book assessing particular homes, 1946-1949; report on the incidence of enuresis (incontinence) in homes, 1946-1950; publicity material mainly created at the time of the centenary and on other children's charities, 1951-1981; careers and apprenticeship literature, 1938-1954; photographs and negatives of students and buildings, 1938-1939 (Boxes 60-62); psychological testing materials including test cards displaying words and pictures, [1958] (Boxes 63-69).

The records of the Pestalozzi Village Trust, 1948-1989, comprise typescript notes compiled by Millicent Coleman, who served on its governing Council. These consist mainly of Council minutes and supporting material, 1948-1989; Committee minutes including Finance and Management Committees, 1953-1985; Annual Reports and Accounts, 1961-1974; policy reports on the development and strategic direction of the Village, 1959-1973; correspondence with Millicent Coleman regarding Trust business and liaison with the National Children's Home, 1953-1985.

Typescript copy of the memoirs of Harry Gooding Field entitled 'Adventures in Finance', 21 Oct 1942, detailing his accountancy career working in Canada, the United States, Malaysia and Singapore, with copies of birth, marriage and death certificate and other official documents relating to Harry Gooding Field.

Papers relating to Gibbs' early career, 1917-1927, including typescript copies [1972] of combat reports written by Gibbs, 17 Sqn, Macedonia, 1917-1918; typescript notes by Gibbs entitled 'Service experiences', 1926; typescript Staff College essay entitled 'Leadership and morale', 1927. Nine typescript texts of lectures by Gibbs, 1948-1972, on the RAF in World War Two, post war airpower, India and the Indian Air Force and the North Atlantic Treaty Organisation (NATO), also 'Air power in modern war', by MRAF Arthur William Tedder, 1st Baron Tedder of Glenguin, 1947. Papers relating to Gibbs' career in the RAF, 1945-1954, including correspondence and typescript notes by Gp Capt I C Bird on the war efforts of India, South Africa and the Colonies [1948]; letter andgraph by Wg Cdr J D Warne, dated 1949, on numbers of sorties flown and losses suffered by the Luftwaffe and the RAF during the Battle of Britain, 1940; typescript copies of correspondence between Gibbs and Adm Louis Francis Albert Victor Nicholas Mountbatten, 1st Earl Mountbatten of Burma, Commander-in-Chief, Mediterranean, 1953; typescript report by Gibbs entitled 'Report on the progressand the policy problems of the Indian Air Force', 1954. Papers and correspondence, 1955-1984, including typescript article by Gibbs entitled 'The lessons of Skybolt, Britain's new defence plans', with letter from Sir Hugh (Nicholas) Linstead MP, 1963; typescript memorandum by MRAF Sir John Cotesworth Slessor entitled 'Integration of the Services within the new defence organisation', 1964;correspondence with Dr G Vincent Orange, History Department, University of Canterbury, Christchurch, New Zealand, dated 1982, concerning research for A biography of Air Chief Marshal Sir Keith Park GCB, KBE, MC, DFC, DCL (Methuen, London, 1984), with copy of letter from ACM Sir Keith Rodney Park, Air Commander-in-Chief, South East Asia to MRAF Sir Charles Frederick Algernon Portal, Chief of the Air Staff, relating to the possible replacement of Gibbs as Chief Air Staff Officer, Supreme Headquarters South East Asia Command [1945]. Copies of Gibbs' letters to the press, 1955-1982, relating chiefly to defence issues, service pensions, capital punishment, immigration and Rhodesia. Publications and articles, 1928-1961, including copy of Air Ministry Air Publication 1308 entitled 'A selection of lectures and essays from the work of officers attending the fifth course at the Royal Air Force Staff College, 1926-1927', (HMSO, London, 1928), including article by Gibbs 'Lecture on fighter squadrons in air defence'; article by Gibbs 'Aircraft types and strategical mobility', Journal of the Royal Air Force College, 1930; booklet by Gen Sir Archibald Percival Wavell entitled 'Generals and Generalship' (reprinted from The Times, London, 1941); three editions of Impact magazine, subtitled 'US Tactical air power in Europe', May 1945, 'Strategic air victory in Europe', Jul 1945, and 'Air victory over Japan', Sep-Oct 1945; restricted pamphlet by MRAF Hugh Montague Trenchard, 1st Viscount Trenchard of Wolfeton, entitled 'Air power', 1946; restricted pamphlet by US Gen Carl A Spaatz entitled 'American views on air power', 1947; article by ACM Sir Keith Rodney Park entitled 'Background to the Blitz, from Hawker Siddeley Review, Dec 1951; article by Gibbs 'The development of defence in NATO's second decade', The British Survey, Feb 1959; article entitled 'Maintaining the deterrent in the future', by Gibbs, The Aeroplane, Mar 1961.

The collection covers Pyman's career from 1937 until 1963 when he suffered a severe stroke which forced his retirement in 1964. The earliest papers date from Pyman's work with the Royal Tank Cadre in converting the 17/21 Lancers from a cavalry to an armoured regiment. There are also papers from Pyman's period as an instructor at the Staff College in Quetta, India, 1939-1941. Pyman was involved in the World War Two campaigns by the 8 Army in the Western Desert, in 1941 as General Staff Officer with 7 Armoured Div, 30 Corps and in 1942-1943 as Commander of the 3 Royal Tank Regiment, 10 Armoured Div, 30 Corps. The papers consist mostly of Pyman's assessments of lessons learned from the ongoing campaigns particularly with regard to tanks and armoured units. In 1944-1945 Pyman was Brigidier General Staff, 30 Corps, 2 Army in the Normandy landings and the invasion of Northern Europe, with particular responsibility for organisation and planning of the Rhine crossing and advance to the Baltic. This is reflected in the papers which largely consist of planning studies and reports for the operations involved, this section also contains maps used in the campaign. Pyman's next appointment was as Chief of General Staff, Allied Land Forces, South East Asia, 1945-1946 which is documented by a series of diaries which reflect the tasks faced by Pyman in this command including dealing with the build up of tension between newly liberated former colonies keen to assert their right for independence and the former colonial powers such as France and Netherlands. Pyman spent 1946-1949 as Chief of Staff, Middle East Land Forces and kept monthly diaries which form the bulk of this section of the collection. The diary entries and additional papers reflect the debate over policy in the Middle East in the British Government and Military command, they include detail on the British withdrawal from Greece, the problem of illegal Jewish immigrants and their internment in Cyprus, the end of the British mandate in Palestine and the the effect of this on relations between Britain with Egypt and the other Arab states and the subsequent Arab Israeli conflict. This section of the collection also contains correspondence between Pyman and Maj Gen Sir Miles Christopher Dempsey on personal matters and on the Middle East. There are also papers from Pyman's work at the Ministry of Supply as Director General of Fighting Vehicles, 1951-1953, Director of Weapons Development, War Office, 1955-1956 mostly brief diary entries and lecture texts. Pyman was also General Officer Commanding, British Army on the Rhine, 1953-1955 and General Officer Commanding, 1 British Corps, 1956-1958 and the papers relating to these commands consist mostly of lectures, reports and directives reflecting his interest in armoured divisions and training. There are some papers, mostly personal correspondence and press cuttings, from Pyman's final command as Commander-in-Chief Allied Forces Northern Europe in North Atlantic Treaty Organisation (NATO). The collection also contains correspondence relating to Pyman's role as Colonel Commandant of the Royal Tank Regiment and The Royal Armoured Corps and a series of letters covering the reorganisation of the Berks and Westminster Dragoons, of which he was Honorary Colonel. The rest of the collection consists of diaries, correspondence, speeches, writings including the draft copy and papers relating to his autobiography, some preparatory work on a history of the 2 Army and reference works. The collection also includes the Boer War diaries and other papers of Col James Redmond Patrick Gordon who commanded the 1 Cavalry Bde of the South African Field Force 1900-1901 which were given to Pyman by a friend.