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The correspondence largely contains letters sent to the Secretary of King’s College London concerning all aspects of the business of the College and its related bodies including King’s College School, 1831- 1908; the Ladies Department of King’s College, subsequently King’s College for Women, from 1885; and some aspects of the business of King’s College Hospital, 1839-1909, relating to new appointments and resignations as well as letters from the Secretaries of the Hospital - mainly regarding decisions of the Committee of Management.

The series contains letters from subscribers to the College regarding their donations, shareholdings or the nomination of prospective students; letters from staff include applications for posts, the content of syllabuses, appeals to College Council for funds for improved facilities, the names of prize and scholarship winners, requests to take in boarders, hold posts at other organisations, and resignations; letters from students and parents include general enquiries about the College, applications for enrolment, requests to remove pupils from King’s College School, applications from prize-winners for their prizes, applications for the AKC (Associateship of King’s College) the College’s own academic award, requests for the refunding of fees; letters from the College Architect regarding the building and later redevelopments of the Strand site; letters from businesses connected to the College including those who supplied equipment and groceries to the College and estimates from contractors for building work; letters from external bodies and individuals regarding the use of rooms in the College, donations and gifts to the College museums and Departments; correspondence relating to schools in union with the College; and papers regarding College Commemoration Days and the Gilbart Lectures on Banking.

The series is remarkably complete until the late 1890s. With the appointment of Walter Smith in 1895 came the introduction of a modern filing system (see KAS/GC, AC and AD) although bundles continued to be used on occasion until 1919. A few letters in the collection post date 1919, but these are largely related to loans of letters for historical research.