The Office of the Principal supports the academic and administrative work of the College's chief officer. Ronald Montagu Burrows was Principal of King's from 1913 until 1920, following a distinguished career as Professor of Greek at University College, Cardiff (1898-1908) and the University of Manchester (1908-1913). The collection comprises Principal Ronald Montagu Burrows' office files including correspondence, memoranda and accounts, 1912-1920. These include correspondence relating specifically to the impact on the College of World War One, including war grants, War Office classes, war-work by staff, lists of student casualties, the Officer Training Corps (OTC), the special constabulary, War Relief Council, erection of a war memorial, lists of refugee students, their status, examinations taken and the hospitality they enjoyed; reports and correspondence relating to the teaching and assessment of individual subjects or departments including Anatomy, Chemistry, Chinese, Day Training, Engineering, Law, Modern Greek, Portuguese, Russian, Spanish and Theology, 1913-1919; correspondence relating to scholarships, studentships and medals, 1913-1917; correspondence on staff, notably academic appointments and pensions, and the establishment of new chairs, 1913-1918; correspondence relating to public lectures, 1913-1918; correspondence concerning Egyptian students at King's including lists of names, 1914-1915; correspondence and accounts of King's College for Women including the transference of many of its functions to King's College in the Strand, 1915-1917; correspondence relating to the Westminster Training College, Horseferry Road, 1913-1917; typescript accounts of the Plantanes Hall of Residence [King's College Hospital, Denmark Hill], 1913-1915; estimated accounts of King's College London, 1913-1919; incomplete examination pass lists, 1914-1918; framed photograph of Eleutherios Venizelos, Greek Statesman, [1913-1920].

Chelsea College of Science and Technology and Chelsea College Department of the Humanities student and other records, 1958-1983. This class of material contains some student information on BSc and visiting BA undergraduate and DCC (Diploma of Chelsea College) students, 1967-1983. BSc and DCC information typically includes name, course work including aggregate marks, percentage marks, letter grading, honour points, degree, class and comments. The remainder of the collection comprises correspondence, accounts and financial data, timetables and printed programmes and handouts. This includes general correspondence on the administration of the College, with the Registry and notably concerning resource allocation, 1958-1983; correspondence with other College departments, 1958-1978; staff correspondence, 1968-1983; selective summary of Senate minutes, 1967-1981; accounts books, 1961-1982; finance yearly estimates, 1959-1983; administrative proposals and submissions relating to the strategic development of the College, 1959-1982; Humanities' Annual Reports, 1958-1982; examination question papers and related correspondence, 1969-1983; handouts describing the course content of the Diploma in Modern Social and Cultural Studies, 1969-1982, and visiting undergraduate BA programmes, 1975-1982; syllabuses and notices of liberal and arts events, 1958-1981.

The records of the Chemistry Department, King's College London, comprise minutes, correspondence, cash books, student progress reports, laboratory experimental reports, syllabuses, photographs and publications, 1906-1985. These notably include committee and staff minutes, 1952-1982; correspondence relating to staff appointments and pay awards, 1951-1972; correspondence and photographs relating to alumni, 1924-1979; grant application reports for proposed projects, 1976-1980; working party reports of a joint committee of chemistry departments in the University of London, 1979-1982; cash books, 1923-1931, 1959-1967; mark books for students' laboratory experiments, 1919-1960; laboratory reports of chemistry experiments carried out by students, 1906-1983; syllabuses and course unit synopses, 1960-1985; photographs of students, staff and laboratories, [1910-1980]; printed publications on chemical laboratory apparatus, 1947-1953; student files, 1946-1986 (Ref: KDCH/FP); student record cards, [1910-1928] (Ref: KDCH/FPC); class files, 1972-1984 (Ref: KDCH/1-9); and tutee reports, 1976-1979 (Ref: KDCH/10-13).