The papers of Kathleen and Millicent Coleman comprise three classes of material: the private papers of the sisters and the Coleman family, 1842-1957; records relating to the National Children's Home, 1935-1981 largely CLOSED; and the Pestalozzi Village Trust, 1948-1989. Personal papers include a diary and pharmacopoeias, correspondence, examination certificates, photographs and printed books, 1842-1957, notably including a detailed manuscript medical diary describing life on board ship and a medical practice in Africa, 1842-1844, probably compiled by John Albert Sidney Coleman, grandfather of Kathleen and Millicent Coleman; pharmacopoeias containing remedies and prescriptions, with printed pharmacopoeias, compiled by Mark Coleman and others, reflecting the transition of the Coleman family business from patent remedies to modern pharmacy, 1851-1894; correspondence with Kathleen and Millicent Coleman, mainly descriptions of daily life in the National Children's Home and describing psychological testing of the children, 1927-1948 (CLOSED); family correspondence and legal documents including letting agreements and deeds of partnership, the will of Mathew Coleman, the sisters' great uncle, and relating to their father and his career, letters containing family news and gossip, 1845-1928; examination certificates and prize lists relating to the education of Kathleen and Millicent Coleman, 1922-1933; photographs of the Coleman family during the 1890s, during World War One and of Kathleen and Millicent Coleman on holiday, [1928], of Lady Eleanor Holles School, 1921-1933, group photographs of students and staff in King's College London Department of History, 1929-1955, photographs of various National Children's Home establishments, 1934-1957; a small collection of printed books concerned with the history, customs and government of London and the Home Counties, [1945-1985] (Boxes 70-74, now on open access in the Archive reading room).

The CLOSED records of the National Children's Home, 1935-1981, notably comprising Vocational Guidance Record Sheets, consisting of files on individual children that included intelligence test results, memory tests and individual comments, arranged in alphabetical order, 1938-1964 (Boxes 1-23); test results and evaluations of named children for tests organised by the National Institute of Industrial Psychology including the Porteus Maze Test and scoring sheets, 1957-1960 (Boxes 24-28); psychological evaluations of children at different branches of the children's home, notably in Cardiff, Harpenden, Nottingham and Glasgow, including individual test results and assessments with broad statistics and educational recommendations by visitors, 1942-1963 (Boxes 29-40); pupil record cards containing biographical information, aptitude tests and psychological test results for children at various homes, [1948-1960] (Boxes 41-42); material relating to the Brentwood College of Education including a working party on syllabuses, staff lists, the relationship with the University of London Institute of Education, manuscript notes and some psychological test results of children engaged in the so-called Gifted Child Study, 1971-1974 (Boxes 43-44); material relating to vocational aptitude and the placement of older children in trades and professions such as the armed forces and Civil Service, notably including psychologists' reports, 1935-1965 (Boxes 45-56); questionnaires of 18 year-old former residents conducted in 1954-1956 (Box 57); material relating to European refugees resident in the NCH including named children and correspondence with the Central Committee for Refugees, 1942-1949 (Boxes 58-59); general correspondence with Millicent Coleman relating to local authorities, staff and the emigration of children to Australia, 1951-1962; manuscript visitation report book assessing particular homes, 1946-1949; report on the incidence of enuresis (incontinence) in homes, 1946-1950; publicity material mainly created at the time of the centenary and on other children's charities, 1951-1981; careers and apprenticeship literature, 1938-1954; photographs and negatives of students and buildings, 1938-1939 (Boxes 60-62); psychological testing materials including test cards displaying words and pictures, [1958] (Boxes 63-69).

The records of the Pestalozzi Village Trust, 1948-1989, comprise typescript notes compiled by Millicent Coleman, who served on its governing Council. These consist mainly of Council minutes and supporting material, 1948-1989; Committee minutes including Finance and Management Committees, 1953-1985; Annual Reports and Accounts, 1961-1974; policy reports on the development and strategic direction of the Village, 1959-1973; correspondence with Millicent Coleman regarding Trust business and liaison with the National Children's Home, 1953-1985.

King's College London student entrance papers, 1831-1935 (Ref: KA/E). These comprise first admissions, Senior Department, 1831-1846 (Ref: KA/E/A), General Literature and Science, 1846-1906 (Ref: KA/E/A), Arts, 1907-1935 (Ref: KA/E/A), Applied Science, 1846-1889 (Ref: KA/E/E), Engineering, 1889-1934 (Ref: KA/E/E), Science, 1901-1935 (Ref: KA/E/S), Medical, 1831-1935 (Ref: KA/E/M), Medical Intercollegiate, 1905-1935 (Ref: KA/E/MI), Theology, 1846-1935 (Ref: KA/E/T), Laws, 1911-1935 (Ref: KA/E/L), Evening Classes, 1855-1916 (Ref: KA/E/EV), Evening Regular, 1916-1934 (Ref: KA/E/EV), Evening Occasional, 1916-1935 (Ref: KA/E/EO), Occasional, 1832-1914 (Ref: KA/E/O), Day Occasional, 1912-1935 (Ref: KA/E/DO), Theological Occasional, 1911-1935 (Ref: KA/E/TO), Matriculation/Preliminary Class, 1898-1935 (Ref: KA/E/P), Military Department, 1849-1859 (Ref: KA/E/ML), Choral Exhibitioners, 1849-1856 (Ref: KA/E/CH), Civil Service Department, 1853-1855 (Ref: KA/E/CI), Day Training Department, 1890-1905 (Ref: KA/E/DT), State Medical Department, 1891-1925 (Ref: KA/E/SM), Bacteriological Department, Public Health and Bacteriology, 1892-1925 (Ref: KA/E/BA), King's Scholars, 1906-1913 (Ref: KA/E/SC), War Refugee students, 1914-1919 (Ref: KA/E/REF), American students, 1919 (Ref: KA/E/AEF), War Service students, 1919-1921 (Ref: KA/E/WAR). This series constitutes the principal source of information on students until 1918. Information typically contained includes name, address, date of entry, age on entering the College, name and address of parent/guardian, major subject(s), fees, previous education. The Occasional and Evening series are generally limited to name, address and course studied. This series is supported by an original set of indices.

The series continues with admission papers for women, 1921-1976 (Ref: KA/E/F), admission papers for men in the Arts Faculty, 1923-1963 (Ref: KA/E/MA), admission papers for men in the Science Faculty, 1923-1976 (Ref: KA/E/MS), admission papers for men and women in the Science Faculty, 1974-1982 (Ref: KA/E/MFS), postgraduate admission forms, 1980-1985 (Ref: KA/E/PG). Faculties and departments covered within the admission papers for women include Arts, Sciences, Law, Journalism, Medicine, Theology, Education, Evening Classes and two-year degree courses. Admission papers for men also include two-year degree courses, Indian students and some non-registered students. The admission papers for men and women in the Science Faculty consist of photocopies of Universities Central Council on Admissions (UCCA) forms and cover the departments of Biology, Botany and Zoology. Information typically contained in this series includes name, age last birthday, name and address of parent/guardian, term-time residence, nationality, previous education, names of referees, course of study proposed, exams passed, scholarships, date of proposed entry, fees, tutor appointments, correspondence, declaration to abide by College rules, and where applicable, National Service number.