The papers of Kathleen and Millicent Coleman comprise three classes of material: the private papers of the sisters and the Coleman family, 1842-1957; records relating to the National Children's Home, 1935-1981 largely CLOSED; and the Pestalozzi Village Trust, 1948-1989. Personal papers include a diary and pharmacopoeias, correspondence, examination certificates, photographs and printed books, 1842-1957, notably including a detailed manuscript medical diary describing life on board ship and a medical practice in Africa, 1842-1844, probably compiled by John Albert Sidney Coleman, grandfather of Kathleen and Millicent Coleman; pharmacopoeias containing remedies and prescriptions, with printed pharmacopoeias, compiled by Mark Coleman and others, reflecting the transition of the Coleman family business from patent remedies to modern pharmacy, 1851-1894; correspondence with Kathleen and Millicent Coleman, mainly descriptions of daily life in the National Children's Home and describing psychological testing of the children, 1927-1948 (CLOSED); family correspondence and legal documents including letting agreements and deeds of partnership, the will of Mathew Coleman, the sisters' great uncle, and relating to their father and his career, letters containing family news and gossip, 1845-1928; examination certificates and prize lists relating to the education of Kathleen and Millicent Coleman, 1922-1933; photographs of the Coleman family during the 1890s, during World War One and of Kathleen and Millicent Coleman on holiday, [1928], of Lady Eleanor Holles School, 1921-1933, group photographs of students and staff in King's College London Department of History, 1929-1955, photographs of various National Children's Home establishments, 1934-1957; a small collection of printed books concerned with the history, customs and government of London and the Home Counties, [1945-1985] (Boxes 70-74, now on open access in the Archive reading room).

The CLOSED records of the National Children's Home, 1935-1981, notably comprising Vocational Guidance Record Sheets, consisting of files on individual children that included intelligence test results, memory tests and individual comments, arranged in alphabetical order, 1938-1964 (Boxes 1-23); test results and evaluations of named children for tests organised by the National Institute of Industrial Psychology including the Porteus Maze Test and scoring sheets, 1957-1960 (Boxes 24-28); psychological evaluations of children at different branches of the children's home, notably in Cardiff, Harpenden, Nottingham and Glasgow, including individual test results and assessments with broad statistics and educational recommendations by visitors, 1942-1963 (Boxes 29-40); pupil record cards containing biographical information, aptitude tests and psychological test results for children at various homes, [1948-1960] (Boxes 41-42); material relating to the Brentwood College of Education including a working party on syllabuses, staff lists, the relationship with the University of London Institute of Education, manuscript notes and some psychological test results of children engaged in the so-called Gifted Child Study, 1971-1974 (Boxes 43-44); material relating to vocational aptitude and the placement of older children in trades and professions such as the armed forces and Civil Service, notably including psychologists' reports, 1935-1965 (Boxes 45-56); questionnaires of 18 year-old former residents conducted in 1954-1956 (Box 57); material relating to European refugees resident in the NCH including named children and correspondence with the Central Committee for Refugees, 1942-1949 (Boxes 58-59); general correspondence with Millicent Coleman relating to local authorities, staff and the emigration of children to Australia, 1951-1962; manuscript visitation report book assessing particular homes, 1946-1949; report on the incidence of enuresis (incontinence) in homes, 1946-1950; publicity material mainly created at the time of the centenary and on other children's charities, 1951-1981; careers and apprenticeship literature, 1938-1954; photographs and negatives of students and buildings, 1938-1939 (Boxes 60-62); psychological testing materials including test cards displaying words and pictures, [1958] (Boxes 63-69).

The records of the Pestalozzi Village Trust, 1948-1989, comprise typescript notes compiled by Millicent Coleman, who served on its governing Council. These consist mainly of Council minutes and supporting material, 1948-1989; Committee minutes including Finance and Management Committees, 1953-1985; Annual Reports and Accounts, 1961-1974; policy reports on the development and strategic direction of the Village, 1959-1973; correspondence with Millicent Coleman regarding Trust business and liaison with the National Children's Home, 1953-1985.

The Soviet Estimate: US Analysis of the Soviet Union, 1947-1991 is a themed microfilm collection which presents an integrated record of US intelligence estimates and studies relating to Soviet strategic projections, military capabilities, science and technology, economics and internal politics, 1946-1991. The estimates and studies were produced either collectively as national intelligence products or by individual agencies, and include contributions from the US Central Intelligence Agency (CIA); the Director of Central Intelligence; the US Defense Intelligence Agency; and, the US State Department. The collection includes CIA and British Secret Intelligence Service debriefing transcripts of former Soviet Gavnoye Razvedyvatelnoye Upravleniye (GRU), Chief Intelligence Directorate, Soviet General Staff, operative Oleg V Penkovskii, relating to Soviet military organisation and plans for nuclear war, Soviet nuclear targets and deployments in Europe, missile technology and launch sites, Soviet military personnel, the capture of Capt Francis Gary Powers, US Air Force U-2 High Altitude Reconnaissance Aircraft pilot, 1 May 1960, profiles of Soviet military officers, locations of Soviet nuclear weapons tests, Soviet intelligence organisations and Soviet chemical and biological weapons programs, Soviet development and deployment of Inter-Continental Ballistic Missiles (ICBMs), positions of Soviet divisions in East Germany, and the Berlin Crisis (1958- 1962), 20 Apr-14 Oct 1961; yearly US estimates of Soviet strategic capabilities, 1947- 1983, including the 'missile gap' National Intelligence Estimates, 1957-1961; detailed estimates of the Soviet space program, including National Intelligence Estimates (NIEs) relating to lunar exploration, manned space flight, reconnaissance satellites, space exploration, space weapons and weapons development, 1962-1967; US Air Force report entitled 'A History of Strategic Arms Competition: Volume 3, A Handbook of Selected Soviet Weapons and Space Systems', including data relating to Soviet air to surface missiles (AS), Tupolev bomber aircraft, M-4 / Mya-4 / 2M Myasishchev ('Bison') aircraft, space weapons, communication satellites, electronic intelligence capabilities, surface to surface (SS) theatre missiles and ICBMs, Intermediate Range Ballistic Missiles (IRBMs), Submarine-Launched Ballistic Missiles (SLBMs), Jun 1976; US intelligence community experiment in competitive analysis conducted by the CIA 'B Team' relating to US misperceptions of Soviet strategic objectives and offensive and defensive forces, Dec 1976; report from the US Department of State entitled 'History of the Strategic Arms Competition 1945-1972, parts 1 and 2', including detailed surveys and analyses of Soviet and US decision making on nuclear forces, force deployments, and nuclear strategies, Mar 1981; Special National Intelligence Estimate relating to Soviet support for international terrorism and revolutionary activities, including mention of arms transfers, military training, political violence, and terrorist activities in Africa, Asia, Europe, Latin America and the Middle East, May 1981; reports from the CIA concerning Soviet perspectives on research and development in energy-directed weapons and involvement in space weapons and Strategic Defense Initiative (SDI) research, 1985; National Intelligence Estimates relating to General Secretary of the Soviet Communist Party Mikhail Sergeyevich Gorbachev's prospects for reforming the Soviet economic and political system, including mention of his economic agenda and its implications for the Soviet military program, the dynamics of Soviet civil-military relations, the impact of reforms on labour production, health, standards of living and technological development, and the rise of civil unrest and nationalism in the Soviet Union, 1985- 1989; CIA report concerning the probabilities of a coup d'etat in the Soviet Union and the growing influence of Chairman of the Russian Republic Supreme Soviet, Boris Nikolayevich Yeltsin, May 1991.